Discovery of (1S,2S)-Cyclohexane-1,2-diamine

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Time Dependent Structural Evolution of Porous Organic Cage CC3

Herein we followed the structural evolution of a prototypical type of porous organic cage, CC3, as a function of synthesis time. Three distinctive crystal formation stages were identified: at short synthesis times, a rapid crystal growth stage in which amorphous agglomerates transformed into larger irregular particles was observed. At intermediate synthesis times, a decrease in crystal size over time was observed presumably due to crystal fragmentation, redissolution, and/or homogeneous nucleation. Finally, at longer synthesis times, a regrowth process was observed in which particles coalesced through Ostwald ripening leading to a continuous increase in crystal size. Molecular simulation studies, based on the construction of in silico CC3 models and simulation of XRD patterns and nitrogen isotherms, confirm the samples at different synthesis times to be a mixture of CC3alpha and CC3-amorphous phases. The CC3alpha phase is found to contract at different synthesis times, and the amorphous phase is found to essentially disappear at the longest synthesis time. Nitrogen and carbon dioxide adsorption properties of these CC3 phases were evaluated, and were highly dependent on synthesis time.

I hope this article can help some friends in scientific research. I am very proud of our efforts over the past few months and hope to 21436-03-3, help many people in the next few years., 21436-03-3

Reference£º
Chiral Catalysts,
Chiral catalysts – SlideShare